Title

Analytical Calculation of Two-dimensional Spectra

Document Type

Article

Publication Date

3-17-2015

Organizational Units

College of Natual Science and Mathematics, Physics and Astronomy

Abstract

We demonstrate an analytical calculation of two-dimensional (2D) coherent spectra of electronic or vibrational resonances. Starting with the solution to the optical Bloch equations for a two-level system in the 2D time domain, we show that a fully analytical 2D Fourier transform can be performed if the projection-slice and Fourier-shift theorems of Fourier transforms are applied. Results can be fit to experimental 2D coherent spectra of resonances with arbitrary inhomogeneity.

Publication Statement

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