Date of Award

8-1-2018

Document Type

Masters Thesis

Degree Name

M.S.

Organizational Unit

Physics and Astronomy

First Advisor

Mark Siemens, Ph.D.

Second Advisor

Kingshuk Gosh

Third Advisor

Gareth Eaton

Keywords

Dynamics, Femtosecond, Laser, Raman, Ultrafast, Vibrations

Abstract

Femtosecond Stimulated Raman Spectroscopy (FSRS) is a ultrafast spectroscopy technique first implemented by chemists to understand isomerization and other ultrafast molecular morphology changes by resolving vibrational dynamics[1, 2, 3]. FSRS has an unparalleled temporal and spectral resolution [4, 1, 5, 6] that arises as a result of a clever combination of picosecond and femtosecond pulses. However, despite this capability, FSRS has yet to be applied to modern materials in condensed matter physics. This thesis explores the design and implementation of FSRS to study two-dimensional materials in order to measure their quantum confined vibrational dynamics on utlrafast time scales.

Publication Statement

Copyright is held by the author. User is responsible for all copyright compliance.

Rights Holder

Daniel Hammerland

Provenance

Received from ProQuest

File Format

application/pdf

Language

en

File Size

111 p.

Discipline

Condensed matter physics



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